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Total synthesis of (–)-tubingensin B enabled by the strategic use of an aryne cyclization

16:56 EDT 19 Jun 2017 | Nature Publishing

The total synthesis of tubingensin B — an indole diterpenoid that bears a daunting chemical structure — has now been achieved. The design and evolution of this succinct total synthesis underscores the utility of long-avoided aryne intermediates for the introduction of structural motifs that have conventionally been viewed as challenging.

Original Article: Total synthesis of (–)-tubingensin B enabled by the strategic use of an aryne cyclization

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