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The sorption behavior of selenite onto the Tamusu clay from a preselected high-level radioactive waste disposal site in Inner Mongolia, China, was first investigated in simulated groundwater with high salinity by batch sorption experiments under aerobic/anaerobic conditions. The results demonstrated that the K values rapidly decreased and then remained steady in the pH range of 2.0-8.0. However, selenite sorption was promoted when pH exceeded 8.0, which might be attributed to the coprecipitation between Ca and SeO. Besides, the change trend of the K values as functions of various parameters was not affected by oxygen. The sorption kinetics and isotherms could be well fitted by the pseudo-second-order kinetic model and the Freundlich model for both aerobic and anaerobic conditions, and the calculated thermodynamic parameters (△G and △H) suggested that the selenite sorption process was a spontaneous and endothermic process. Additionally, the XPS results revealed that Se(IV) could be reduced to Se (0) only in anaerobic conditions and that the different amounts of Fe on the clay surface led to the discrepancy of the Se(IV) K values under aerobic and anaerobic conditions even in high-salt simulated groundwater. Overall, our findings in this study are significant in regards to the retardation of selenite on the host rock under high salinity conditions.
This article was published in the following journal.
Name: Journal of environmental radioactivity
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Selenious acid, disodium salt. It is used therapeutically to supply the trace element selenium.
Liquid water present beneath the surface of the earth.
Contamination of bodies of water (such as LAKES; RIVERS; SEAS; and GROUNDWATER.)
Elimination of toxic or biologically active substances from body fluids by interaction with a sorbent medium. The types of media include absorbents, adsorbents, ion-exchange materials, and complexing agents. Detoxification can be extracorporeal (hemodialysis, hemofiltration, hemoperfusion, plasmapheresis), or occur inside the body (enterosorption, peritoneal dialysis).
A change in cardiovascular function resulting in a reduction in BLOOD VOLUME, and reflex DIURESIS. It occurs frequently after actual or simulated WEIGHTLESSNESS.