Nickel phosphate nanorod-enhanced polyethylene oxide-based composite polymer electrolytes for solid-state lithium batteries.

07:00 EST 7th January 2020 | BioPortfolio

Summary of "Nickel phosphate nanorod-enhanced polyethylene oxide-based composite polymer electrolytes for solid-state lithium batteries."

Solid-state electrolytes with high ionic conductivity, large electrochemical window, and excellent stability with lithium electrode are needed for high-energy solid-state lithium batteries. In this work, a novel polyethylene oxide (PEO)-Lithium bis(trifluoromethylsulphonyl)imide (LiTFSI)-nanocomposite-based polymer electrolyte was prepared by using nickel phosphate (VSB-5) nanorods as the filler. The ionic conductivity of the obtained PEO-LiTFSI-3%VSB-5 solid polymer electrolyte was found to be as high as 4.83 × 10 S·cm at 30 °C and electrochemically stable up to about 4.13 V versus Li/Li. The enhanced ionic conductivity was attributed to the reduced crystallinity of the PEO and the interaction between VSB and 5 and PEO-LiTFSI. In addition, the solid polymer electrolyte exhibited improved compatibility to the lithium metal anode with excellent suppression of lithium dendrites. The assembled LiFePO/Li battery with the PEO-LiTFSI-3%VSB-5 solid polymer electrolyte showed better rate performance and higher cyclic stability than the PEO-LiTFSI electrolyte. It is demonstrated that this new solid polymer hybrid should be a promising electrolyte applied in solid state batteries with lithium metal electrode.


Journal Details

This article was published in the following journal.

Name: Journal of colloid and interface science
ISSN: 1095-7103
Pages: 110-118


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